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Yes, you can upgrade most with SSD now but there is a major latency problem with larger SSD's. Latency can double or even triple with larger drives, which is why they are rarely used. If your issue is that users would tear down a company owned notebook and install a bigger SSD, you have problems WELL beyond the scope of users adding unwanted files. Many companies, for the last couple of decades, set forth and enforce company policies, it might be a good idea for your organization too.

The relevant comment you added was "Chrome OS would be the last option I'd choose"

Seeing as that fits the topic of discussion, can you share your reasons?